Osment expanded her repertoire into pop music and more recently alternative/indie rock where she has recorded teen pop hits like "I Don't Think About It," "If I Didn't Have You" alongside her Hannah Montana co-star Mitchel Musso, and most recently "Once Upon a Dream."

She is recording her debut album, which features several songs written by her,[6] due for release in June 2010,[7] on Wind-up Records[8] where she recently signed. Emily collaborated on the album with Tom Higgenson of the Plain White T's, Toby Gad, Mandi Perkins and Eve 6's Max Collins & Tony Fagenson. [9][10] The first single from the album, "Let's Be Friends," premiered on June 7, 2010. [11]